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1 article(s) from Seghetti, Francesca

Selectivity in multiple multicomponent reactions: types and synthetic applications

Ouldouz Ghashghaei,
Francesca Seghetti and
Rodolfo Lavilla

Beilstein J. Org. Chem. 2019, 15, 521–534, doi:10.3762/bjoc.15.46

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Graphical Abstract

Scheme 1: Selectivity levels found in multiple multicomponent reactions. I) Innate selectivity; II) sequentia...

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Scheme 2: Indiscriminate double Ugi MCR upon pyridine-2,6-dicarboxylic acid.

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Scheme 3: Representative examples of MCR-polymer synthesis. A) Biginelli HTS of polymers; B) Passerini;- C) U...

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Scheme 4: Concept of multicomponent macrocyclization.

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Scheme 5: Supramolecular structures out of MMCR macrocyclizations.

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Scheme 6: Macrocyclization by MMCRs. A) Staudinger MCR; B) boronic-imine MCR.

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Scheme 7: Selective Sequential MMCRs. A and B) MCRs involving terephthalaldehyde; C) Multiple GBB processes w...

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Scheme 8: Biased substrates for selective MMCRs.

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Scheme 9: The Union concept. A) Asinger–Ugi combination; B) Passerini–Ugi/azide from anthranilic acid; C) Pas...

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Scheme 10: Relevant examples of consecutive MCRs exploiting the Union Concept. A) Petasis-Ugi combination; B) ...

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Scheme 11: Selective MMCRs featuring FGs with distinct reactivity along the sequence. A) Synthesis of aminomet...

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Scheme 12: High order MMCRs. A) Ugi/Ugi–Smiles 7C combination; B) imidazoline-N-cyanomethylamide-Ugi union lea...

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Scheme 13: Consecutive Ugi 4CR-deprotection–Ugi 4CR strategy towards A) PNA oligomers and B) peptidic tetrazol...

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Scheme 14: Sequential Ugi 4CR-deprotection access to cyclopeptoids.

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Scheme 15: Stepwise access to 6-aminopenicillanic acid derivative through an Asinger, deprotection, Joullié ap...

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Scheme 16: A triple MCR-deprotection approach affording anticancer peptidomimetics.

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Review

Published 21 Feb 2019

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