Beilstein J. Nanotechnol.2018,9, 1770–1781, doi:10.3762/bjnano.9.168
University of Technology, Tianjin 300384, China 10.3762/bjnano.9.168 Abstract Novel hexagonal nanoplates (NPLs) comprised of mesoporous carbon containing imbedded magnetic Co nanoparticles (CoAl2O4 phase) are prepared through direct carbonization of polydopamine (PDA)-coated CoAl layered double hydroxide
: absorbent regeneration; CoAl layered double hydroxide; efficient adsorbent; hexagonal nanoplates; magnetic nanoparticles; polydopamine; Introduction
Nanocomposites with unique electronic, mechanical, magnetic, and physicochemical properties have gained much attention because of their large specific surface
be used as a type of carbon precursor with a high carbonization yield even at a high carbonization temperature [20]. More notably, it can self-polymerize under weak basic conditions at room temperature [21] and form a uniform coating [22] on almost any surface. The obtained polydopamine (PDA)-coated
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Scheme 1:
Schematic illustration of the formation process of the hexagonal magnetic mesoporous nanoplates.
Beilstein J. Nanotechnol.2018,9, 591–601, doi:10.3762/bjnano.9.55
magnetic actuators. However, the tendency of magnetite particles to migrate within the matrix and, ultimately, escape from the aerogel structure, remains a technological challenge. In this article we show that coating magnetite particles with polydopamine anchors them on graphene oxide defects
, immobilizing the particles in the matrix and, at the same time, improving the aerogel structure. Polydopamine coating does not affect the magnetic properties of magnetite particles, making the fabricated materials promising for industrial applications.
Keywords: aerogel; composite; Fe3O4 nanoparticles
; polydopamine; reduced graphene oxide; Introduction
Preparation of hybrid aerogels based on two-dimensional carbon nanomaterials with unique physicochemical properties is among the most popular recent nanotechnological trends [1]. With this respect, graphene oxide (GO) is one of the most exploited aerogel
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Figure 1:
SEM micrographs of rGO (a,d), rGO-Fe3O4 (b,e) and rGO-PDA@Fe3O4 (c,f) aerogel structures.