Nitrogen-vacancy centers in diamond for nanoscale magnetic resonance imaging applications

• Alberto Boretti,
• Lorenzo Rosa,
• Jonathan Blackledge and
• Stefania Castelletto

Beilstein J. Nanotechnol. 2019, 10, 2128–2151, doi:10.3762/bjnano.10.207

• technique that can dramatically increase the signal-to-noise ratio (SNR) in traditional MRI. The method is being applied to small injectable endogenous molecules, which can be used to monitor transient in vivo metabolic events in real time. Among all methodologies, the emergence of hyperpolarized 13C

Review of advanced sensor devices employing nanoarchitectonics concepts

• Katsuhiko Ariga,
• Tatsuyuki Makita,
• Masato Ito,
• Taizo Mori,
• Shun Watanabe and
• Jun Takeya

Beilstein J. Nanotechnol. 2019, 10, 2014–2030, doi:10.3762/bjnano.10.198

• solution. Ultrasensitive sensors for mercury ions were prepared by Li et al. who engineered suspended atomically thin black phosphorus between the source and drain electrodes [94]. Due to the avoidance of substrate scattering, the sensors with bridged black phosphorus exhibit a much improved signal-to

• -noise ratio in mercury ion detection with a detection limit of 0.01 ppb and a very short detection time constant of 3 s. This nanoarchitectonic design can maximize the intrinsic potential of black phosphorus and other materials. Sensors for physical conditions Not limited to particular chemicals, the

Optimization and performance of nitrogen-doped carbon dots as a color conversion layer for white-LED applications

• Tugrul Guner,
• Hurriyet Yuce,
• Didem Tascioglu,
• Eren Simsek,
• Umut Savaci,
• Aziz Genc,
• Servet Turan and
• Mustafa M. Demir

Beilstein J. Nanotechnol. 2019, 10, 2004–2013, doi:10.3762/bjnano.10.197

• ratio approaches unity while the overall emission reaches the lowest level, the resulting LER is reduced again to only 196 lm/W. The reason for this decrease may be the very low PL intensity (blue line in Figure 3a), which results in a low signal-to-noise ratio (S/N). The low S/N possibly causes an

Magnetic properties of biofunctionalized iron oxide nanoparticles as magnetic resonance imaging contrast agents

• Natalia E. Gervits,
• Andrey A. Gippius,
• Alexey V. Tkachev,
• Evgeniy I. Demikhov,
• Sergey S. Starchikov,
• Igor S. Lyubutin,
• Alexander L. Vasiliev,
• Vladimir P. Chekhonin,
• Maxim A. Abakumov,
• Alevtina S. Semkina and
• Alexander G. Mazhuga

Beilstein J. Nanotechnol. 2019, 10, 1964–1972, doi:10.3762/bjnano.10.193

• core–shell structure iron oxide nanoparticles of the same size has already been described and calculated based on magnetic measurements. In the HSA-coated sample, we also succeeded to observe the ZF-NMR signal, despite the very low iron content per unit volume and the resulting low signal-to-noise

• ratio. As evident from Figure 9, at least at 4.2 K, there is no significant difference in the NMR spectra of the HSA-coated and uncoated samples. Conclusion In this work, we studied and compared the structural and magnetic properties of uncoated and functionalized (HSA-coated) iron oxide nanoparticles

Development of a new hybrid approach combining AFM and SEM for the nanoparticle dimensional metrology

• Loïc Crouzier,
• Alexandra Delvallée,
• Sébastien Ducourtieux,
• Laurent Devoille,
• Guillaume Noircler,
• Christian Ulysse,
• Olivier Taché,
• Elodie Barruet,
• Christophe Tromas and
• Nicolas Feltin

Beilstein J. Nanotechnol. 2019, 10, 1523–1536, doi:10.3762/bjnano.10.150

• to take the full width at half maximum (FWHM) [19]. The profile FWHM depends on the accelerating voltage (or EHT) corresponding to the primary electron energy as shown in Figure 1. Above 4 kV, the signal-to-noise ratio, corresponding to the difference in grey level between the NP and the substrate

Fabrication of phase masks from amorphous carbon thin films for electron-beam shaping

• Lukas Grünewald,
• Dagmar Gerthsen and
• Simon Hettler

Beilstein J. Nanotechnol. 2019, 10, 1290–1302, doi:10.3762/bjnano.10.128

• the central lobe [26]. In practice, this may result in a reduced signal-to-noise ratio and a compromise has to be found between a large kρ and sufficient intensity in the central lobe [25]. While the radial beam profile in form of a Bessel function is preserved upon propagation up to zmax, the

Fe₃O₄ nanoparticles as a saturable absorber for giant chirped pulse generation

• Ji-Shu Liu,
• Xiao-Hui Li,
• Abdul Qyyum,
• Yi-Xuan Guo,
• Tong Chai,
• Hua Xu and
• Jie Jiang

Beilstein J. Nanotechnol. 2019, 10, 1065–1072, doi:10.3762/bjnano.10.107

• analyzer (Rohde & Schwarz FSC6) is used to measure the signal-to-noise ratio of the pulse. There are many methods that can be employed for the synthesis of NPs, such as sol–gel, sol–hydrothermal, co-precipitate, or dry methods. Due to the homogeneity and the versatility of the product, a sol–hydrothermal

• smooth shape with a center wavelength of 1560.6 nm and 3 dB bandwidth of 0.8 nm at a pump power of 245.2 mW [41]. As shown in Figure 5b and 5c, the RPR of 4.63 MHz corresponds to a laser cavity length of about 43 m, which is verified by the time interval of the output pulse train. The signal-to-noise

• ratio (SNR) of 63 dB indicates that the fiber laser operates in a stable state. In Figure 5c, the evolution diagram of SNR intensity with the change of RPR (range about 0–40 MHz) is given, and the repetition interval between them is also 4.63 MHz. The output pulse can be well fit with a Gaussian profile

Influence of dielectric layer thickness and roughness on topographic effects in magnetic force microscopy

• Alexander Krivcov,
• Jasmin Ehrler,
• Marc Fuhrmann,
• Tanja Junkers and
• Hildegard Möbius

Beilstein J. Nanotechnol. 2019, 10, 1056–1064, doi:10.3762/bjnano.10.106

• increase the signal-to-noise ratio. The resolution of the images is 254 measuring points per line, and the scan speed is 0.9 Hz. The force gradient is detected by phase shifts in interleave mode. A magnetic ASYMFM-HM tip was used for all measurements in order to assure a high magnetic sensitivity. The

Correlation of surface-enhanced Raman scattering (SERS) with the surface density of gold nanoparticles: evaluation of the critical number of SERS tags for a detectable signal

• Vincenzo Amendola

Beilstein J. Nanotechnol. 2019, 10, 1016–1023, doi:10.3762/bjnano.10.102

• linear response, it was found that 10 SERS AuNTs inside the probed area are required. These findings indicate that a better signal-to-noise ratio requires high-magnification optics, while linearity versus tag number can be improved by using low-magnification optics or a high tag density. In general the

• inside the probed area is required to obtain a linear response, that is, on the order of 10 tags. Overall, these results suggest that a better signal-to-noise ratio requires optics with a high numerical aperture, while linearity versus tags number is improved by using low-magnification optics. However

Fabrication of silver nanoisland films by pulsed laser deposition for surface-enhanced Raman spectroscopy

• Bogusław Budner,
• Mariusz Kuźma,
• Barbara Nasiłowska,
• Bartosz Bartosewicz,
• Malwina Liszewska and
• Bartłomiej J. Jankiewicz

Beilstein J. Nanotechnol. 2019, 10, 882–893, doi:10.3762/bjnano.10.89

• single point were 1 s, 5 s and 0.5 s for 532 nm, 633 nm, and 785 nm excitation wavelengths, respectively. The measurement parameters were adjusted to different nominal output power values of the lasers to obtain a good signal-to-noise ratio for a single measuring point. SERS measurements were made for

• the EF of the Raman signal, the Raman measurements of the pMA adsorbed on the surface of the platinum film were also done. Compared to SERS substrates, obtaining a spectrum with the appropriate signal-to-noise ratio required increasing the laser power and extended measurement time. For the 532 nm

Commercial polycarbonate track-etched membranes as substrates for low-cost optical sensors

• Paula Martínez-Pérez and
• Jaime García-Rupérez

Beilstein J. Nanotechnol. 2019, 10, 677–683, doi:10.3762/bjnano.10.67

• the spectrum was notably noisy, with a signal-to-noise ratio (SNR) value of 3.52 (see Figure 2b). All these issues are disadvantageous for the future employment of these membranes as optical sensing structures for two reasons. First, the noise can hide tiny displacements of the spectra that could

Review of time-resolved non-contact electrostatic force microscopy techniques with applications to ionic transport measurements

• Aaron Mascaro,
• Yoichi Miyahara,
• Tyler Enright,
• Omur E. Dagdeviren and
• Peter Grütter

Beilstein J. Nanotechnol. 2019, 10, 617–633, doi:10.3762/bjnano.10.62

• larger number of averages, the same signal-to-noise ratio can be achieved, however the cantilever resonance frequency will ultimately determine the minimum τPLL. Empirically we have found that the minimum PLL response time achievable is τPLLmin ≈ 10 × 1/f0. The highest resonance frequency cantilevers

• sample is metallic (see discussion below). The authors also derived similar ratios for both the sub-resonant and super-resonant schemes, allowing them to directly compare the time resolution and signal-to-noise ratio of each. Validation measurement As a validation measurement, they applied electrical

• the IMP spacing (δ). The signal-to-noise ratio is significantly lower in this case, requiring a much smaller value of δ and, in turn, longer averaging times. Note that since the time resolution is proportional to δ (Equations 15 and 16 in [20]), using a smaller δ values actually results in better time

Quantification and coupling of the electromagnetic and chemical contributions in surface-enhanced Raman scattering

• Yarong Su,
• Yuanzhen Shi,
• Ping Wang,
• Jinglei Du,
• Markus B. Raschke and
• Lin Pang

Beilstein J. Nanotechnol. 2019, 10, 549–556, doi:10.3762/bjnano.10.56

• ). Correspondingly, we observe similar CE values, independent of excitation fluence, within the range of powers investigated, limited by the signal-to-noise-ratio for low powers, and thermal effects at high powers. The dashed lines are linear fits to the data with CE = 1.9 × 10−9 × (Power)4 + 13 for 785 nm and CE

Site-controlled formation of single Si nanocrystals in a buried SiO₂ matrix using ion beam mixing

• Xiaomo Xu,
• Thomas Prüfer,
• Daniel Wolf,
• Hans-Jürgen Engelmann,
• Lothar Bischoff,
• René Hübner,
• Karl-Heinz Heinig,
• Wolfhard Möller,
• Stefan Facsko,
• Johannes von Borany and
• Gregor Hlawacek

Beilstein J. Nanotechnol. 2018, 9, 2883–2892, doi:10.3762/bjnano.9.267

• , compared to the 25 eV SiO2 plasmon-loss peak, due to its better signal-to-noise ratio. The NC diameter was evaluated using Otsu thresholding [38] in Fiji [39]. The calculation of the projected Si thickness d (Equation 7) from the Si plasmon-loss filtered images was performed in the following way. The

Charged particle single nanometre manufacturing

• Philip D. Prewett,
• Cornelis W. Hagen,
• Claudia Lenk,
• Steve Lenk,
• Marcus Kaestner,
• Tzvetan Ivanov,
• Ahmad Ahmad,
• Ivo W. Rangelow,
• Xiaoqing Shi,
• Stuart A. Boden,
• Alex P. G. Robinson,
• Dongxu Yang,
• Sangeetha Hari,
• Marijke Scotuzzi and
• Ejaz Huq

Beilstein J. Nanotechnol. 2018, 9, 2855–2882, doi:10.3762/bjnano.9.266

• the lines were broken at a line dose of 0.04 nC·cm−1, which is equivalent to 25 ions per nanometre, i.e., a signal-to-noise ratio of 5:1. The line discontinuity is caused by shot noise producing missing pixels. Thus 6 nm represents the current limit of 1:1 dense features using SHIBL to expose HM-01A

Effective sensor properties and sensitivity considerations of a dynamic co-resonantly coupled cantilever sensor

• Julia Körner

Beilstein J. Nanotechnol. 2018, 9, 2546–2560, doi:10.3762/bjnano.9.237

• . However, the co-resonantly coupled system’s frequency shift response to an external interaction is only one aspect. The other equally important aspect is the detectability, i.e., how well the oscillatory state of a dynamic-mode cantilever sensor can be detected. That is limited by the signal-to-noise

• ratio (SNR) for frequency, amplitude and phase measurements. It mainly depends on the cantilever’s quality factor which directly influences the phase noise and resolution of the resonance peak [19]. With decreasing cantilever dimensions, the quality factor usually decreases, hence, detectability

Intrinsic ultrasmall nanoscale silicon turns n-/p-type with SiO₂/Si₃N₄-coating

• Dirk König,
• Daniel Hiller,
• Noël Wilck,
• Birger Berghoff,
• Merlin Müller,
• Sangeeta Thakur,
• Giovanni Di Santo,
• Luca Petaccia,
• Joachim Mayer,
• Sean Smith and
• Joachim Knoch

Beilstein J. Nanotechnol. 2018, 9, 2255–2264, doi:10.3762/bjnano.9.210

• respective energy values as extracted from the spectra (dashed lines). The light green and cyan lines show the background fit of the amorphous Si3N4-matrix. The lower signal-to-noise ratio for Si-NWells embedded in Si3N4 as compared to SiO2 is comprehensively evaluated and discussed in Supporting Information

Filling nanopipettes with apertures smaller than 50 nm: dynamic microdistillation

• Evelyne Salançon and
• Bernard Tinland

Beilstein J. Nanotechnol. 2018, 9, 2181–2187, doi:10.3762/bjnano.9.204

• small and large angles, would therefore be highly desirable. It would help to improve the spatial resolution in scanning conductance experiments, in optimizing the signal-to-noise ratio during single-molecule delivery and in straining long-molecule stretching during translocation. Small nanopipette

Know your full potential: Quantitative Kelvin probe force microscopy on nanoscale electrical devices

• Amelie Axt,
• Ilka M. Hermes,
• Victor W. Bergmann,
• Niklas Tausendpfund and
• Stefan A. L. Weber

Beilstein J. Nanotechnol. 2018, 9, 1809–1819, doi:10.3762/bjnano.9.172

• this mode as AM-KPFM off resonance (AM off res). This mode is implemented on older AFM systems, where the auxiliary lock-ins were limited in terms of the maximum frequency they could measure. The biggest drawback of this method is the lower signal-to-noise ratio (SNR) resulting from the off-resonance

Sulfur-, nitrogen- and platinum-doped titania thin films with high catalytic efficiency under visible-light illumination

• Boštjan Žener,
• Lev Matoh,
• Giorgio Carraro,
• Bojan Miljević and
• Romana Cerc Korošec

Beilstein J. Nanotechnol. 2018, 9, 1629–1640, doi:10.3762/bjnano.9.155

• high signal-to-noise ratio, preventing an unambiguous attribution of the peak tailing at higher/lower energies, which are attributed to the absorption of other nitrogen species [46]. On the other hand, the presence of Ti–N bonds can be clearly ruled out [46][48]. In the sample S3_N0.5+1%Pt, the Pt 4f7

Cathodoluminescence as a probe of the optical properties of resonant apertures in a metallic film

• Kalpana Singh,
• Evgeniy Panchenko,
• Babak Nasr,
• Amelia Liu,
• Lukas Wesemann,
• Timothy J. Davis and
• Ann Roberts

Beilstein J. Nanotechnol. 2018, 9, 1491–1500, doi:10.3762/bjnano.9.140

• ] and enhanced coupling to plasmonic cavities by emitters such as quantum dots [36]. One way to enhance the signal-to-noise ratio of transmission measurements is to study the collective optical properties of an array of apertures, choosing the periodicity to minimize both the effects of diffraction and

Excitation of nonradiating magnetic anapole states with azimuthally polarized vector beams

• Aristeidis G. Lamprianidis and
• Andrey E. Miroshnichenko

Beilstein J. Nanotechnol. 2018, 9, 1478–1490, doi:10.3762/bjnano.9.139

• useful applications in biosensing, i.e., in the detection of molecules that interact strongly once exposed to magnetic field hotspots, which nanoparticles in a magnetic anapole state can offer in their near field. Moreover, the signal-to-noise ratio of an MRI machine, that is defined as the ratio of the

Room-temperature single-photon emitters in titanium dioxide optical defects

• Kelvin Chung,
• Yu H. Leung,
• Chap H. To,
• Aleksandra B. Djurišić and
• Snjezana Tomljenovic-Hanic

Beilstein J. Nanotechnol. 2018, 9, 1085–1094, doi:10.3762/bjnano.9.100

• , this is a unique feature to the nanopowder and is not evident in the other single emitters presented in this study. Figure 6b is the spectrum of the defect, which shows red emission with a peak around 629 nm. The low signal-to-noise ratio was counteracted by increasing the exposure time at each step

Lyapunov estimation for high-speed demodulation in multifrequency atomic force microscopy

• David M. Harcombe,
• Michael G. Ruppert,
• Michael R. P. Ragazzon and
• Andrew J. Fleming

Beilstein J. Nanotechnol. 2018, 9, 490–498, doi:10.3762/bjnano.9.47

• , they provide an increased signal-to-noise ratio. The MF-LYAP can be seen to perform comparably to the LIA when tuned to similar measurement bandwidth settings. When imaging with higher harmonics, the off-mode rejection of each channel was tuned to suppress the large fundamental frequency. Imaging a PS

The nanofluidic confinement apparatus: studying confinement-dependent nanoparticle behavior and diffusion

• Stefan Fringes,
• Felix Holzner and
• Armin W. Knoll

Beilstein J. Nanotechnol. 2018, 9, 301–310, doi:10.3762/bjnano.9.30

• 35,000 detected positions obtained from 7 immobilized particles. This precision is in agreement with simulated particles [26] with a similar signal-to-noise ratio (SNR) of ≈20. We like to point out that we measure the same SNR using raw images similar to that in Figure 2b, but for moving particles we can